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lambertellols a and b, novel 3,4-dihydronaphthalen-1(2h)-ones with spiro-butenolide produced by lambertella sp.1346.[structure: see text] lambertella sp. 1346 was found to produce lambertellols a (1) and b (2) carrying a novel dihydronaphthalen-1(2h)-ones with spiro-1-furan-2(5'h)-one. the spiro-lactone ring moiety of both 1 and 2 were easily migrated to afford lambertellin, a known metabolite of lambertella corni-maris. the absolute stereochemistry of these compounds was established on the basis of cd spectrum after chemical derivatization.200414723517
stimulation of the biosynthesis of the antibiotics lambertellols by the mycoparasitic fungus lambertella corni-maris under the acidic conditions produced by its host fungus in vitro.the filamentous fungus, lambertella corni-maris (l. corni-maris), a mycoparasite on monilinia fructigena, produces the antibiotics, lambertellols a (1), b (2), and lambertellin (3), in a substantial amounts under acidic conditions, whereas these antibiotics were hardly detected when the fungus was cultured on a potato-sucrose (ps) medium without added acids. our investigations also revealed that the host, m. fructigena, changed its surroundings into acidic conditions, suggesting that the acidic ...200717485857
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